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Hello @robna, congratz with the FAIR Data Prize! That's how I found this repo ;)
I saw your spectra and was thinking if you might be interested in a package that pre-processes and can deconvolute parts of these type of spectra. I wrote this package for that https://github.com/MyPyDavid/raman-fitting.
Are you pursuing the de-convolution of these spectra?
Please let me know if it is of interest.

ref https://microplastix-specdb.streamlit.app/
Example plots in raman-fitting:
https://github.com/MyPyDavid/raman-fitting/blob/main/examples/fitting_Model_1st_6peaks%2BSi.png
https://github.com/MyPyDavid/raman-fitting/blob/main/examples/raw_data.png
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